Here is a KB link to one way you can dynamically control the contents of one dropdown based on the values set in another using CurretnCellShowingDropDown.
http://www.syncfusion.com/Support/article.aspx?id=567
Here is a sample
that does it in a slightly different manner using grid.Model,QueryCellInfo.
How are you trying to do it? If you cannot use one of the above techniques, can you postt a sample project showing what you are trying to do?