Hi Darran,
Thank you for your interest in syncfusion products.
We have analyzed your requirement of "Bind a Dictionary to Grid Data Control's Item Source" and this is possible to achieve in our Grid Data Control. We have prepared a sample based on this and please find the sample under the following location.
Sample:
http://www.syncfusion.com/uploads/redirect.aspx?&team=support&file=DictionaryBinding-906059462.zipNote: This sample shows an simple dictionary binding and also please let us know if this helps.
Regards,
Ramesh