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Hi Ralf Steigele,
Thank you for using Syncfusion products.
It is possible to set colors for data labels with the following code snippet. Kindly follow the code snippets and let us know if it meets your requirement.
Dim chart As IChart = workbook.Charts(0)
chart.Series(0).DataPoints(0).DataLabels.Color = ExcelKnownColors.Red
chart.Series(0).DataPoints(1).DataLabels.Color = ExcelKnownColors.Green
chart.Series(0).DataPoints(2).DataLabels.Color = ExcelKnownColors.Blue
chart.Series(0).DataPoints(3).DataLabels.Color = ExcelKnownColors.Yellow
We have also provided a sample to illustrate this, which can be downloaded from the following link.
Sample Link : ChartDataPoints.zip