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Hi,
I know you can add items to SfPicker in XAML using:
<syncPicker:SfPicker x:Name="Picker" HeaderText="Select Item" PickerMode="Default" BackgroundColor="Transparent" HeaderBackgroundColor="DodgerBlue" SelectedItemTextColor="#003768"
UnSelectedItemTextColor="Gray" SelectedItemFontSize="38" UnSelectedItemFontSize="35" ShowHeader="true" >
<syncPicker:SfPicker.ItemsSource>
<itemCollection:List x:TypeArguments="x:String">
<x:String>Male</x:String>
<x:String>Female</x:String>
<x:String>Feedback</x:String>
<x:String>Contacts</x:String>
<x:String>Comment</x:String>
<x:String>General</x:String>
</itemCollection:List>
</syncPicker:SfPicker.ItemsSource>
</syncPicker:SfPicker>
<Item Text="Male" Value="M" Image="male.png" />
<Item Text="Feale" Value="F" Image="female.png" />